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Tuning of the active phase structure and hydrofining performance of alumina-supported tri-metallic WMoNi

Shufeng Shan, Haiyan Liu, Gang Shi, Xiaojun Bao

《化学科学与工程前沿（英文）》 2018年 第12卷 第1期   页码 59-69 doi: 10.1007/s11705-017-1686-3

摘要： The effects of phosphorus on the structure and hydrofining performance of tri-metallic WMoNi/Al O catalysts prepared with W/Mo-based hybrid precursor nanocrystals were investigated. The incorporation of phosphorus weakened the metal-support interactions (MSIs) and facilitated the formation of more synergetic NiWMoS phases with higher stacks. Catalytic tests using a fluid catalytic cracking diesel fuel showed that the changes in the MSIs and the morphology of the active phases had a more positive effect on the hydrodenitrogenation activity than on the hydrodesulfurization activity. In contrast, when phosphorus was incorporated into a tri-metallic WMoNiP/Al O catalyst prepared by a conventional incipient impregnation method, the MSIs decreased causing aggregation of the metal species which resulted in poorer hydrofining performance of the catalyst. These results show that incorporating phosphorus into a WMoNi/Al O catalyst can finely tune the structure of the active phase to enhance the hydrogenation and hydrodenitrogenation activity of the resulting tri-metallic catalyst.

关键词： fluid catalytic cracking diesel     hydrofining performance     WMoNiP/Al2O3     synergetic effect and structure of NiWMoS phases    

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Influence of HS and NH on biogas dry reforming using Ni catalyst: a study on single and synergetic effect

《环境科学与工程前沿（英文）》 2023年 第17卷 第3期 doi: 10.1007/s11783-023-1632-1

摘要：

● NH3 in biogas had a slight inhibitory effect on dry reforming.

关键词： Biogas     Dry reforming     Sulfur poisoning     Ammonia     Synergetic effect     Hydrogen    

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Toxic effects of wastewater from various phases of monosodium glutamate production on seed germination

LIU Rui, ZHOU Qixing, ZHANG Lanying, GUO Hao

《环境科学与工程前沿（英文）》 2007年 第1卷 第1期   页码 114-119 doi: 10.1007/s11783-007-0021-5

摘要： To make a comprehensive assessment on monosodium glutamate (MSG) wastewater pollution, a pollution exposure experiment was carried out on the seed germination and root elongation of wheat, Chinese cabbage and tomato by using the wastewater discharged from different processing phases of MSG production. The results showed that there were significantly positive linear relationships between the inhibitory rates of wheat seed germination and root elongation and the COD of the mother liquor scraps. The toxicity of MSG wastewater to the test crops was in the order of tomato > Chinese cabbage > wheat, indicating that tomato was the most sensitive to the wastewater, and could be considered as an ideal toxic bioindicator. The half-effect concentrations (IC) based on the seed germination and root elongation of the test crops exposed to the wastewater discharged from various processing phases of MSG production was 22.0 32 432 and 17.3 3320 mg/L, respectively.

关键词： monosodium glutamate     different     inhibitory     pollution exposure     half-effect    

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Effect of counter current gas phase on liquid film

Shujuan LUO, Huaizhi LI, Weiyang FEI, Yundong WANG

《化学科学与工程前沿（英文）》 2009年 第3卷 第2期   页码 135-137 doi: 10.1007/s11705-009-0129-1

摘要： Liquid film flow is very important in many industrial applications. However, there are few reports about its characteristics on structured packings. Therefore, in this paper, liquid film phenomena were investigated experimentally to exploit new approaches for intensifying the performance of the structured packings. All experiments were performed at room temperature. Water and air were the working fluids. The effect of counter current gas phase on the liquid film was taken into consideration. A high speed camera, a non-intrusive measurement technique, was used. It is shown that both liquid and gas phases have strong effects on film characteristics. In the present work, liquid film width increased by 57% because of increasing liquid flow rate, while it decreased by 25% resulting from the counter current gas phase.

关键词： counter current     liquid film     two phases     structured packings    

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Enhanced performance of oxygen vacancies on CO adsorption and activation over different phases of ZrO

《能源前沿（英文）》 2023年 第17卷 第4期   页码 545-554 doi: 10.1007/s11708-023-0867-7

摘要： The effect of oxygen vacancies on the adsorption and activation of CO2 on the surface of different phases of ZrO2 is investigated by density functional theory (DFT) calculations. The calculations show that the oxygen vacancies contribute greatly to both the adsorption and activation of CO2. The adsorption energy of CO2 on the c-ZrO2, t-ZrO2 and, m-ZrO2 surfaces is enhanced to 5, 4, and 3 folds with the help of oxygen vacancies, respectively. Moreover, the energy barrier of CO2 dissociation on the defective surfaces of c-ZrO2, t-ZrO2, and m-ZrO2 is reduced to 1/2, 1/4, and 1/5 of the perfect surface with the assistance of oxygen vacancies. Furthermore, the activation of CO2 on the ZrO2 surface where oxygen vacancies are present, and changes from an endothermic reaction to an exothermic reaction. This finding demonstrates that the presence of oxygen vacancies promotes the activation of CO2 both kinetically and thermodynamically. These results could provide guidance for the high-efficient utilization of CO2 at an atomic scale.

关键词： CO2 activation     oxygen vacancies     ZrO2     different phases    

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Toxic effect of sodium perfluorononyloxy-benzenesulfonate on in aerobic denitrification, cell structure

《环境科学与工程前沿（英文）》 2021年 第15卷 第5期 doi: 10.1007/s11783-021-1391-9

摘要：

• OBS inhibited the growth of P. stutzeri and destroyed its structure.

关键词： Sodium perfluorononyloxy-benzenesulfonate     Aerobic denitrification     Pseudomonas stutzeri     Ecotoxicity     ROS     Persist organic pollutants     Toxicity     Denitrification     Microbiology    

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Optimising the oil phases of aluminium hydrogel-stabilised emulsions for stable, safe and efficient vaccine

《化学科学与工程前沿（英文）》 2022年 第16卷 第6期   页码 973-984 doi: 10.1007/s11705-021-2123-1

摘要： To increase antibody secretion and dose sparing, squalene-in-water aluminium hydrogel (alum)-stabilised emulsions (ASEs) have been developed, which offer increased surface areas and cellular interactions for higher antigen loading and enhanced immune responses. Nevertheless, the squalene (oil) in previous attempts suffered from limited oxidation resistance, thus, safety and stability were compromised. From a clinical translational perspective, it is imperative to screen the optimal oils for enhanced emulsion adjuvants. Here, because of the varying oleic to linoleic acid ratio, soybean oil, peanut oil, and olive oil were utilised as oil phases in the preparation of aluminium hydrogel-stabilised squalene-in-water emulsions, which were then screened for their stability and immunogenicity. Additionally, the underlying mechanisms of oil phases and emulsion stability were unravelled, which showed that a higher oleic to linoleic acid ratio increased anti-oxidative capabilities but reduced the long-term storage stability owing to the relatively low zeta potential of the prepared droplets. As a result, compared with squalene-in-water ASEs, soybean-in-water ASEs exhibited comparable immune responses and enhanced stability. By optimising the oil phase of the emulsion adjuvants, this work may offer an alternative strategy for safe, stable, and effective emulsion adjuvants.

关键词： pickering emulsion     vaccine adjuvant     alum-stabilised emulsion     oleic to linoleic acid ratio     stability    

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重大建设工程技术创新网络协同要素与协同机制分析

王孟钧,刘慧,张镇森,陆洋

《中国工程科学》 2012年 第14卷 第12期   页码 106-112

摘要：

通过文献研究、现场调研以及访谈等方式，认为工程需求、组织、资源、制度是重大建设工程技术创新网络的4个协同要素，构建由合作机制、利益机制、激励机制和评价机制组成的协同机制模型，并论证通过协同机制的有效运行，能够提升重大建设工程技术创新能力和效率。 本研究为建设工程技术创新网络理论研究的组成部分，对建设工程技术创新实践活动以及制定行业技术创新政策具有一定的理论参考价值。

关键词： 重大建设工程     技术创新网络     协同要素     协同机制    

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Synergetic Management Theory for Coal-Based Energy Engineering and the Engineering Practice of Shenhua

Wen Ling

《工程管理前沿（英文）》 2016年 第3卷 第1期   页码 1-8 doi: 10.15302/J-FEM-2016005

摘要： To deal with problems in synergetic development of coal-based energy engineering, this paper, guided by the philosophy of engineering, proposes the synergetic management philosophy of “factors coordination, systems synergy, dynamic optimization and three-dimension planning.” The paper also establishes the synergetic management system characterized by systems factor synergy, resource-environment synergy and systems boundary extension and supported by the “two-wheel driven” management innovation and technological innovation. In addition, the paper presents a multi-objective dynamic optimization model for energy engineering, designed based on Shenhua’s own engineering practice, to analyze Pareto optimal solution in three scenarios: best resource allocation, minimal environmental impact and maximal value creation. This provides important reference to synergetic development strategies and decision-making in engineering management.

关键词： coal-based energy     engineering synergetic management     two-wheel driven innovation     Shenhua engineering    

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Mapping the structure-activity relationship of

Worawan PANPIPAT, Hasene KESKIN, Zheng GUO

《化学科学与工程前沿（英文）》 2015年 第9卷 第1期   页码 105-113 doi: 10.1007/s11705-015-1502-x

摘要： The phase behavior of twelve synthesized -sitosteryl fatty acid esters with acyl moieties with different chain lengths (C2:0-C18:0) and different degrees of unsaturation (C18:1-C18:3) were investigated in pure and mixed Langmuir monolayers with phospholipids. The surface-pressure isotherms showed that short chain -sitosteryl fatty acid esters gave smaller mean molecular areas and had decreased monolayer stability and the long chain steryl esters did not produce collapsed plateaus. All the steryl esters displayed strong condensing effects, but there was a pronounced structural dependency: medium chain esters (C8 and C10) were less efficient than short and long chain esters. Atomic force microscopy imaging demonstrated that monolayers mixed with dipalmitoyl phosphatidylcholine (DPPC) displayed both DPPC-rich and steryl lipid-rich domains. However, the height and area differences between the two phases and the roughness and morphologic patterns were very dependent on the steryl lipid concentrations as well as the length, the degree of unsaturation and the molecular conformations of the acyl segments. These findings not only provide a better understanding of the interactions between phytosteryl hydrophobic derivatives and biomembranes, but also may be of general use for the design and engineering of phytosterol structural derivations for specific food and pharmaceutical applications.

关键词： β-sitosteryl fatty acid esters     dipalmitoyl phosphatidylcholine     Langmuir monolayer     condensing effect     structure-activity relationship    

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Effect of ambient polycyclic aromatic hydrocarbons and nicotine on the structure of Aβ protein

《环境科学与工程前沿（英文）》 2023年 第17卷 第2期 doi: 10.1007/s11783-023-1615-2

摘要：

● B[a]P, nicotine and phenanthrene molecules altered the secondary structure of Aβ42.

关键词： Polycyclic aromatic hydrocarbons     Nicotine     toxicology     Aβ42 peptide     Alzheimer’s disease     Molecular dynamics simulations     Environmental pollution    

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The effect of conservation tillage on crop yield in China

Hongwen LI,Jin HE,Huanwen GAO,Ying CHEN,Zhiqiang ZHANG

《农业科学与工程前沿（英文）》 2015年 第2卷 第2期   页码 179-185 doi: 10.15302/J-FASE-2015058

摘要： Traditional agricultural practices have resulted in decreased soil fertility, shortage of water resources and deterioration of agricultural ecological environment, which are seriously affecting grain production. Conservation tillage (CT) research has been developed and applied in China since the 1960s and 1970s, and a series of development policies have been issued by the Chinese government. Recent research and application have shown that CT has positive effects on crop yields in China. According to the data from the Conservation Tillage Research Center (CTRC), Chinese Ministry of Agriculture (MOA), the mean crop yield increase can be at least 4% in double cropping systems in the North China Plain and 6% in single cropping systems in the dryland areas of North-east and North-west China. Crop yield increase was particularly significant in dryland areas and drought years. The mechanism for the yield increase in CT system can be attributed to enhanced soil water content and improved soil properties. Development strategies have been implemented to accelerate the adoption of CT in China.

关键词： conservation tillage     crop yield     soil structure     development strategies    

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insights into nitrogen and sulfur co-doped carbon nanotubes for effective desulfurization of liquid phases

《环境科学与工程前沿（英文）》 2021年 第15卷 第5期 doi: 10.1007/s11783-021-1397-3

摘要：

• Synthesis of NS-CNTS is used in a high desulfurization performance.

关键词： Dibenzothiophene (DBT)     Tertiary methyl mercaptan     Adsorption     Carbon nano tube (CNT)     Desulfurization     Doping    

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Dynamics of foot-and-mouth disease virus replication in cells at different phases of the cell-division

Claudia DOEL,Zhidong ZHANG,Lise MAZELET,Ryan WATERS,John BASHIRUDDIN

《农业科学与工程前沿（英文）》 2014年 第1卷 第3期   页码 250-257 doi: 10.15302/J-FASE-2014031

摘要： Foot-and-mouth-disease virus (FMDV) replicates in epithelial cells. The restriction of FMDV RNA to the basal cell layer of epithelia suggests a possible link between FMDV replication and the cell status. This paper describes studies in which FMDV infection was investigated in cells that were held at various cell division phases using cell cycle inhibitors. The results suggest that when cells were arrested at the G or G /S phase, high levels of viral RNA were detected by quantitative real-time reverse transcription PCR and viral protein synthesis was observed by specific labeling techniques. In contrast, when cells were arrested at the G /M phase, reduced or no viral RNA synthesis was detected.

关键词： foot-and-mouth disease virus     cell cycle     replication    

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标题 作者 时间 类型 操作

Tuning of the active phase structure and hydrofining performance of alumina-supported tri-metallic WMoNi

Shufeng Shan, Haiyan Liu, Gang Shi, Xiaojun Bao

期刊论文

Influence of HS and NH on biogas dry reforming using Ni catalyst: a study on single and synergetic effect

期刊论文

Toxic effects of wastewater from various phases of monosodium glutamate production on seed germination

LIU Rui, ZHOU Qixing, ZHANG Lanying, GUO Hao

期刊论文

Effect of counter current gas phase on liquid film

Shujuan LUO, Huaizhi LI, Weiyang FEI, Yundong WANG

期刊论文

Enhanced performance of oxygen vacancies on CO adsorption and activation over different phases of ZrO

期刊论文

Toxic effect of sodium perfluorononyloxy-benzenesulfonate on in aerobic denitrification, cell structure

期刊论文

Optimising the oil phases of aluminium hydrogel-stabilised emulsions for stable, safe and efficient vaccine

期刊论文

重大建设工程技术创新网络协同要素与协同机制分析

王孟钧,刘慧,张镇森,陆洋

期刊论文

郑然：The Carbon Emission Reduction Effect of China's Industrial Structure Transformation with Resource

2022年06月10日

会议视频

Synergetic Management Theory for Coal-Based Energy Engineering and the Engineering Practice of Shenhua

Wen Ling

期刊论文

Mapping the structure-activity relationship of

Worawan PANPIPAT, Hasene KESKIN, Zheng GUO

期刊论文

Effect of ambient polycyclic aromatic hydrocarbons and nicotine on the structure of Aβ protein

期刊论文

The effect of conservation tillage on crop yield in China

Hongwen LI,Jin HE,Huanwen GAO,Ying CHEN,Zhiqiang ZHANG

期刊论文

insights into nitrogen and sulfur co-doped carbon nanotubes for effective desulfurization of liquid phases

期刊论文

Dynamics of foot-and-mouth disease virus replication in cells at different phases of the cell-division

Claudia DOEL,Zhidong ZHANG,Lise MAZELET,Ryan WATERS,John BASHIRUDDIN

期刊论文